Contents

Title Page

1 Introduction and Summary of Results

1.1 Summary of risk assessment results

1.2 Organization of this chapter

1.3 What is tritium?

1.4 Why is tritium used at Lawrence Berkeley National Laboratory?

1.5 What are tritium’s radiological characteristics?

1.6 What steps are necessary to assess tritium risk?

1.7 Does the tritium at LBNL escape into the environment?

1.8 How might someone be exposed to tritium from LBNL?

1.9 Is tritium hazardous to human health? What do we know?

1.10 How much radiation are workers exposed to from the NTLF?

1.11 What are the estimated risks due to tritium exposure?

1.12 What is the likelihood that a worker or community member will suffer a health effect as a result of exposure to background natural radiation?

1.13 What are the risks from LBNL tritium to workers near the NTLF?

1.14 What are the risks from LBNL tritium exposure to other LBNL workers and nearby facilities and residences?

1.15 Does LBNL tritium make it risky to live in Berkeley, or to wade or swim in Strawberry Creek or relax along its banks?

1.16 Is it more likely that this study overstates or understates risk?

1.17 Does LBNL tritium pose a significant risk to workers and the community?

1.18 How reliable is this risk assessment?

1.19 Organization of the rest of this report

1.A Annex to Chapter 1

1A.1 Radiological Health Branch, California Department of Health Services

1A.2 Agency for Toxic Substances and Disease Registry

1A.3 US Environmental Protection Agency, Region IX Office in San Francisco

2 Radiation and Tritium Use at the NTLF

2.1 What Is Radiation?

2.2 Tritium

2.2.1 Sources of Environmental Tritium

2.2.2 Health Effects of Tritium

2.2.3 How People Come in Contact with Tritium

2.2.4 Potential Risks

2.3 Tritium Use at the NTLF

2.3.1 Tritium Labeling

2.3.2 Tritium Releases at the NTLF

3 How the Risk Assessment Was Done

3.1 General Approach

3.2 Computer Modeling Used in the Risk Assessment

3.3 Accidents

4 Technical Details

4.1 Overview of the Risk Assessment Process

4.2 Tritium Properties and Sources

4.2.1 Physical and Chemical Properties of Tritium

4.2.2 Sources of Tritium Release in the Environment

4.3 Tritium Releases from the NTLF

4.4 Environmental Distribution of Tritium Releases from the NTLF

4.4.1 Model Structure

4.4.1.1 Steady State Mass Balance Equations

4.4.1.2 Calculating La

4.4.1.3 Calculating Ls

4.4.2 Solutions for the Tritium Inventories

4.4.3 Air Dispersion Model for Zone 3

4.5 Human Contact with Tritium Releases

4.5.1 Intake and Uptake

4.5.2 Exposure Factors

4.5.2.1 Exposure Duration and Averaging Time

4.5.2.2 Anatomical Properties, Inhalation, and Ingestion

4.5.2.3 Activity Patterns and Exposure Times

4.5.2.4 Dermal Uptake from Air

4.5.2.5 Dermal Uptake from Water

4.6 The Relation Between Tritium Exposure, Radiological Dose and Health Effects

4.6.1 Health Risks Associated with Tritium

4.6.2 Tritium Metabolism and Dosimetry

4.6.3 Regulatory Guidance Relevant to Tritium

4.6.4 Risk Factors: The Relation Between Radiological Dose and Health Effects

4.6.4.1 The Risk Factor for Cancer, Rcan
HTO

4.6.4.2 The Risk Factor for Heritable Genetic Effects, Rgen
HTO

4.6.4.3 The Risk Factor for Developmental and Reproductive Effects, Rrep
HTO

4.7 Estimated Health Risks for Tritium Releases from the NTLF

4.7.1 Tritium Concentrations in Air, Water, and Soil of the NTLF Environment

4.7.1.1 Source Term

4.7.1.2 Source Area and Mixing Height of the Atmosphere Near the NTLF

4.7.1.3 Predicted Concentrations in the Vicinity of the NTLF, Zone 1

4.7.1.4 Predicted Concentrations in Zone 2

4.7.1.5 Predicted Concentrations in Zone 3

4.7.2 Generic Calculations of Intake, Uptake, Body Burdens, and Dose

4.7.2.1 Average Intake by Inhalation

4.7.2.2 Average Dermal Uptake

4.7.2.3 Average Intake by Ingestion of Homegrown Foods

4.7.2.4 Average Ingestion Intake of Surface Water During Recreation

4.7.2.5 Total Body Burden of Tritiated Water

4.7.2.6 Estimated Live-Born Infant Body Burden

4.7.2.7 Potential Infant Intake and Body Burden through Breast Feeding

4.7.2.8 Total Dose, Population Risk, and Individual Risk

4.7.3 Estimated Doses and Risks in Zone 1

4.7.4 Estimated Doses and Risks in Zone 2

4.7.5 Estimated Doses and Risks in Zone 3

4.7.6 Step-by-Step Calculations

4.8 Summary and Discussion


APPENDICES

A Two-Compartment Environmental Transport Model for Tritium

A.1 General Issues

A.1.1 Tritium in Air

A.1.2 Tritium in Soil

A.1.3 Tritium in Surface Waters

A.1.4 Tritium Uptake in Biota

A.1.5 Why Only Two Compartments?

A.2 Steady State Mass Balance Equations

A.2.1 Transfer Rate Constants

A.2.2 Solutions for the Compartment Inventories

B Human Anatomical and Intake Factors Used in the Exposure Assessment Calculations

B.1 Body Weight

B.2 Body Surface Area

B.3 Breathing Rate

B.4 Water Ingestion

B.5 Breast-Milk Ingestion

B.6 Ingestion of Homegrown Fruits, Vegetables, and Grains

C Landscape, Climate and Hydrology Parameters

C.1 Wind Speed

C.2 Temperature

C.3 Humidity

C.4 Depth of Soil Compartment

C.5 Moisture Content of Soil

C.6 Precipitation

C.7 Evapotranspiration

C.8 Runoff

C.9 Infiltration to Ground Water

C.10 Rain Scavenging Efficiency

D Evaluating the Potential Legacy of Past Elevated HTO Emissions

E Results of the Risk Assessment Carried Out for NTLF Releases, Using the EPA CAP88 Computer Model

F Validation of the Input Data for Risk Assessment

F.1 Comparison of Risk Assessment Estimates to Measured Air Quality Data

F.2 Comparison of Risk Assessment Estimates to Measured Rain Water Data

F.3 Comparison of Risk Assessment Estimates to Measured Surface Water Data

F.4 Comparison of Risk Assessment Estimates to Measured Soil and Sediment Data

F.5 Comparison of Risk Assessment Estimates to Measured Ground Water Data

F.6 Comparison of Risk Assessment Estimates to Measured Vegetation Data

F.7 Analysis of Urine Data

G Conversion Table for Radiation Units

H Review Comments

I Questions and Answers About Tritium

J Reviewers’ Letters

Glossary of Technical Terms

References


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Chapter 1

Chapter 2

Chapter 3

Chapter 4

Appendices